OSTI Document ID 13483
Local PDF osti/13483.pdf
Title Plutonium speciation, solubilization, and migration in soils. 1998 annual progress report
Creators/
Authors
Haire, R.G. [Oak Ridge National Lab., TN (US)]; Neu, M.; Runde, W. [Los Alamos National Lab., NM (US)]
Publication Date 1998 Jun 01
Description/
Abstract
The DOE is currently conducting cleanup activities at its nuclear weapons development sites, many of which have accumulated plutonium in soils for 50 years. To properly control Pu migration in soils within Federal sites and onto public lands, better evaluate the public risk, and design effective remediation strategies, a fundamental understanding of Pu speciation, transport, and release mechanisms is needed. Key scientific goals include: determine Pu concentrations and speciation at a contaminated DOE site; study the formation, stability, and structural and spectroscopic features of environmentally relevant Pu (III, IV, and V) species; determine the mechanism of interaction between Pu and Mn/Fe minerals and the potential release of Pu via redox cycling; and model the environmental behavior of plutonium. This report summarizes work after seven months of a three-year project. In the first year of this project the authors are focusing on the origin, speciation, and mobility of plutonium at the Rocky Flats Environmental Test Site (RFETS).
OSTI ID 13483
Report Numbers line line docnumall
Document Type Technical Report
Research Organization Los Alamos National Lab., NM (US); Oak Ridge National Lab., TN (US)
Sponsor Organization USDOE Office of Environmental Management (EM), Office of Science and Risk Policy (US)
Bibliographic Source DOEEMSP
Country United States
Language English
Pages/Size 3 pages
System Entry Date 2001 Aug 22
Subject Category Code 11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS; 54 ENVIRONMENTAL SCIENCES
Descriptors PLUTONIUM; DISSOLUTION; RADIONUCLIDE MIGRATION; SOILS; REMEDIAL ACTION; GEOCHEMISTRY; REDOX REACTIONS; MATHEMATICAL MODELS; ROCKY FLATS PLANT
Keywords PROGRESS REPORT; ACTINIDES; CHEMICAL REACTIONS; BIOGEOCHEMISTRY; REMEDIAL ACTION; HIGH-LEVEL RADIOACTIVE WASTES
Availability INIS ; OSTI as DE00013483
Notes PBD: 1 Jun 1998
Reference Numbers EDB-01:101859; TRN: AH200135%%281; INS-US0110738